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I've painted my dreamcast before. I painted it black with blue power buttons. Kinda looks like an R7 dreamcast. Here are a few things I would suggest.
Patience, you gotta have this if you want it to look good
Buy some high grit sand paper like 320 grit or higher to slightly rough up the surface
As far as the type of paint I used enamel spray paint. In addition to that I also bought some sealent to seal the paint after its dried, and you can choose what type of finish you'd like on it, like glossy, semi, or flat.
Buy good masking tape to mask off anything you don't want painted, this is where the patience stuff is really important.
As far as the dreamcast logo, I used a hobby knife and scraped underneath the logo. I used a little super glue when I put it back on and it seems to stay very well.
That should get you started |